Just as admins can add champions to a group, they can remove them.

To begin, from the desired group's page, select which champions you would like to remove on its Members sub-tab. This is done by checking the checkboxes in the leftmost column of those champions' rows. If you would like to remove all listed champions, you can select the checkbox in the leftmost column of the header. It will check off all listed champions.

Once you have selected the champions you would like to remove, select the orange Remove button above the members' information.

A pop-up will appear, asking you to confirm your decision to remove them. You may also add a note to indicate why they have been removed. Select Remove Member to complete the removal.
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The champion has now been removed from your group!

Note: Removing a champion from a group does not necessarily remove them from your Champions list, and it does not delete their account.